You can't do that.
Here's why. The OnLoad event in ASP.NET for a control is fired while the server is building the page (on the web server), but before it sends it to the browser (running on the user's machine).
Code on the web server can't directly call code on the browser computer (which hasn't even got the page yet).
If you just want to hide the control, just do this in your markup:
<asp:Button ID="btnFromCalOpen" runat="server" Text=" > " visible="false" OnClientClick ="ShowCal()" />
Another approach (hidden control doesn't takes up space):
<asp:Button ID="btnFromCalOpen" runat="server" Text=" > " style="display:none;" OnClientClick ="ShowCal()" />
Another approach (hidden control takes up space)
<asp:Button ID="btnFromCalOpen" runat="server" Text=" > " style="visibility:hidden;" OnClientClick ="ShowCal()" />
style
property. While this is CSS still, you'll be able to control it directly with JavaScript